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No, it is generally not possible to use Google Chrome extensions directly on an LG Smart TV. LG Smart TVs run on webOS, which is not compatible with Chrome extensions, as they are designed to work specifically with the Chrome browser on desktop operating systems like Windows, macOS, or Linux.

However, you can access web-based services through the TV's built-in browser or use apps available in the LG Content Store. If you're looking to extend functionality, you might need to find specific apps designed for smart TVs or use a separate device (like a Chromecast, Android TV box, or laptop) to cast Chrome with extensions enabled to your TV.